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生物质化学制氢技术研究进展
Review of hydrogen production from biomass by chemical conversion process

查看参考文献65篇

文摘 可再生生物质制氢是未来氢能的主要来源,涉及到化学制氢和生物制氢.生物质化学制氢技术包括生物质气化、热解、超临界转化等常规热化学法制氢和生物质解聚液相产物的蒸汽重整、水相重整、自热重整和光催化重整制氢等技术.对以上生物质制氢方法进行了综述,对反应条件、反应机理、催化剂使用、技术经济性及各自存在的优缺点进行分类整理与比较.认为生物质气化制氢及热解制氢技术的发展较成熟,可以实现规模化生产,但是制氢的选择性和产氢率不高;生物质液相产物催化重整制氢技术更适合较大规模的集中制氢,转化率和产氢率高,但技术途径复杂.对生物质制氢技术进行了展望.
其他语种文摘 Hydrogen from biomass is considered to be an important future hydrogen supplier. It usually contains chemical and biological conversion. Conventional thermo-chemical conversion covers gasification, pyrolysis and supercritical process,and catalytic reforming includes steam reforming, aqueous-phase reforming, auto-thermal reforming and photocatalytic reforming process using the liquid products derived from biomass depolymerization. These processes that mentioned above were overviewed and their operating conditions, reaction mechanism, catalysts, economic-technical advantages and disadvantages were compared. Gasification or pyrolytic conversion is approaching industrial scale, but hydrogen selectivity and yield are far from satisfactory. Catalytic reforming process of the biomass-derived liquid product may be applicable to scale-up with high hydrogen selectivity and yield, but technological process is still under development. The future developing direction of biomass to hydrogen development was pointed out.
来源 浙江大学学报. 工学版 ,2014,48(7):1318-1328 【核心库】
DOI 10.3785/j.issn.1008-973x.2014.07.025
关键词 生物质 ; 制氢 ; 热化学转化 ; 催化重整
地址

天津大学环境科学与工程学院, 天津, 300072

语种 中文
文献类型 研究性论文
ISSN 1008-973X
学科 能源与动力工程;化学工业
基金 国家973计划 ;  国家自然科学基金资助项目 ;  国家自然科学基金青年基金资助项目
文献收藏号 CSCD:5209316

参考文献 共 65 共4页

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