夜郎湖水库水体不同形态汞的时空分布
Spatial and temporal distribution of mercury species in water in Yelanghu Reservoir.
查看参考文献22篇
文摘
|
于2006年7月(夏季)、2007年1月(冬季)和3月(春季)采集了贵州省夜郞湖水库水样,研究了不同形态汞(总汞、溶解态汞、颗粒态汞)的时空分布特征及其影响因素。结果表明,夏季水体总汞、溶解态汞、颗粒态汞平均含量分别为4.48±2.59、2.37±1.40、2.11±1.86 ng·L-1,均显著高于冬季和春季(P<0.001),而冬春2季不同形态汞含量无明显差异。水质参数悬浮颗粒物(SPM)和硝酸盐(NO-3)与不同形态汞之间均存在显著的正相关关系,表明这些参数对于不同形态汞的季节分布起着重要作用。夏季农业耕作活动相对活跃,表层土壤的扰动增加,雨水冲刷农田土壤,带进大量的外源颗粒物,致使夜郞湖水体夏季总汞水平较高。空间分布表明,夜郞湖水库夏季总汞平均浓度从水库入库河流至大坝方向、出库河流呈现总体下降的分布趋势,但水体各采样剖面没有明显的分布规律。 |
其他语种文摘
|
A study was conducted during July 2006,January 2007 and March 2007 to determine the distribution of mercury species (total Hg (THg),dissolved Hg (DHg),particulate Hg (PHg))and the impacts of some major controlling factors in the Yelanghu Reservoir,Guizhou,China.By comparison,the average concentrations of THg (4.48±2.59 ng·L-1),DHg (2.37±1.40 ng·L-1),PHg (2.11±1.86 ng·L-1)in the summer campaign are significantly higher (P<0.001)than those in the winter and spring campaigns,while no significant differences of concentrations of different mercury species are found between the latter two campaigns.Our investigation revealed that SPM and NO-3 may play an important role in controlling the seasonal distribution of mercury species in the reservoir.It is assumed that higher concentrations of mercury species in the summer could be a result of runoff impact.High runoff volume due to abundant precipitation in the summer carried Hg-containing particulates eroded from the agriculture-dominated watershed into the reservoir.Spatial distribution reveals that mercury concentrations generally decreased from the reservoir inlet to the outlet,while no notable vertical trends were found at each sampling site. |
来源
|
生态学杂志
,2011,30(5):969-975 【核心库】
|
关键词
|
夜郞湖水库
;
总汞
;
时空分布
;
控制因素
|
地址
|
1.
贵州省环境科学研究设计院, 贵州省水污染控制与资源化技术研究重点实验室, 贵阳, 550081
2.
中国科学院地球化学研究所, 环境地球化学国家重点实验室, 贵阳, 550002
|
语种
|
中文 |
文献类型
|
研究性论文 |
ISSN
|
1000-4890 |
学科
|
水产、渔业 |
基金
|
国家自然科学基金重点项目
;
贵州省2008年度科学技术基金项目
|
文献收藏号
|
CSCD:4205884
|
参考文献 共
22
共2页
|
1.
郭艳娜. 乌江流域梯级水库入出库河流中总汞和甲基汞的时空分布.
长江流域资源与环境,2009,18(4):356-360
|
CSCD被引
5
次
|
|
|
|
2.
郭艳娜.
乌江流域不同演化阶段水库汞的输人输出通量研究[博士学位论文],2008
|
CSCD被引
1
次
|
|
|
|
3.
蒋红梅. 蒸馏-乙基化GC-CVAFS法测定天然水体中的甲基汞.
中国环境科学,2004,24(5):568-571
|
CSCD被引
65
次
|
|
|
|
4.
刘继文. 三岔河流域生态现状及污染防治的探索..
环境污染与防治(网络版),2006(3):1-8
|
CSCD被引
1
次
|
|
|
|
5.
石庆. 农业面源污染对贵州省水库影响的初步分析..
贵州水力发电,2007,21(5):15-18
|
CSCD被引
1
次
|
|
|
|
6.
张军方.
乌江流域普定、东风水库汞的分布与质量平衡研究[博士学位论文],2009
|
CSCD被引
2
次
|
|
|
|
7.
朱俊.
水坝拦截对乌江生源要素生物地球化学循环的影响[博士学位论文],2005
|
CSCD被引
2
次
|
|
|
|
8.
Baeyens W. Speciation of mercury in different compartments of the environment..
Trends in Analytical Chemistry,1992,11:245-254
|
CSCD被引
3
次
|
|
|
|
9.
Balogh SJ. Transport of mercury in three contrasting river basins..
Environmental Science & Technology,1998,32:456-462
|
CSCD被引
1
次
|
|
|
|
10.
Bloom NS. Seasonal variability in mercury speciation of Onondaga Lake(New York)..
Water,Air,and Soil Pollution,1990,53:251-265
|
CSCD被引
3
次
|
|
|
|
11.
Bonzongo JC. Mercury levels in surface waters of the Carson river-Lahontan Reservoir system,Nevada:Influence of historic mining activities..
Environmental Pollution,1996,92:193-201
|
CSCD被引
7
次
|
|
|
|
12.
Bonzongo JC. Impact of land use and physieochemical settings on aqueous m ethyl mercury levels in the Mobile Alabama River System..
Ambio,2004,33:328-333
|
CSCD被引
2
次
|
|
|
|
13.
Brigham ME. Methylmercury in flood-control impoundments and natural waters of Northwestern Minnesota,1997-1999..
Water,Air,and Soil Pollution,2002,138:61-78
|
CSCD被引
6
次
|
|
|
|
14.
Cosovic B. Distribution and seasonal variability of organic matter in a small eutrophied salt lake..
Estuarine,Coastal and Shelf Science,2000,51:705-715
|
CSCD被引
1
次
|
|
|
|
15.
Gill GA. Mercury speciation in surface freshwater systems in California and other areas..
Environmental Science & Technology,1990,24:1392-1400
|
CSCD被引
7
次
|
|
|
|
16.
He TR. The impact of eutrophication on the biogeochemical cycling of mercury species in a reservoir:A case study from Hongfeng Reservoir,Guizhou,China..
Environmental Pollution,2008,154:56-67
|
CSCD被引
1
次
|
|
|
|
17.
Lyons WB. Mercury geochemistry of the Scioto River,Ohio:Impact of agriculture and urbanization..
Applied Geochemistry,2006,21:1880-1888
|
CSCD被引
6
次
|
|
|
|
18.
Mason RP. Mercury and methylmercury transport through an urban watershed..
Water Research,1998,32:321-330
|
CSCD被引
7
次
|
|
|
|
19.
Montgomery S. Total dissolved mercury in the water column of several natural and artificial aquatic systems of northern Qu6bec(Canada)..
Canadian Journal of Fisheries and Aquatic Sciences,1995,52:2483-2492
|
CSCD被引
3
次
|
|
|
|
20.
USEPA.
Mercury Study Report to Congress,1997
|
CSCD被引
2
次
|
|
|
|
|