梯级水库修建对乌江甲基汞分布的影响
Effect of Construction of Cascade Reservoirs on the Distribution of Methylmercury in Wujiang River
查看参考文献27篇
文摘
|
采用蒸馏-乙基化结合(GC-CVAFS)法,测定了2006年乌江流域梯级水库系统入、出库河流甲基汞的含量,探讨了其分布特征和时空变化规律以及梯级水库修建对河流甲基汞分布的影响.结果表明:乌江流域梯级水库系统入库河流水体中ρ(总甲基汞)和ρ(溶解态甲基汞)分别为0.07-0.70和0.03-0.16 ng/L;出库河流水体中ρ(总甲基汞)和ρ(溶解态甲基汞)分别为0.10-0.34和0.04-0.26 ng/L.入库河流水体中ρ(总甲基汞)与ρ(悬浮物)有显著的正相关关系,并且丰水期高于枯水期;出库河流水体中ρ(总甲基汞)在夏秋季节显著高于冬春季节.梯级水库的修建使乌江在多个河段的ρ(甲基汞)升高,并且随着水库生态系统的不断演化,下游河流水体中ρ(甲基汞)有升高的可能. |
其他语种文摘
|
Methylmercury concentrations of inflows and outflows in cascade reservoirs in Wujiang River were determined by distillation- ethylation (GC-CVAFS) technique in 2006. The distribution and temporal and spatial variation of methylmercury were discussed. The results were as follows: ρ(total methylmercury) ranged from 0.07 to 0.70 ng/L and ρ(dissolved methylmercury) from 0.03 to 0.16 ng/L in inflows. In outflows ρ(total methylmercury) ranged from 0.10 to 0.34 ng/L and ρ(dissolved methylmercury) from 0.04 to 0.26 ng/L. The obvious positive relationship between ρ( total methylmercury) and ρ ( total suspended matter) was found in inflows, and ρ ( total methylmercury) in high flow was higher than that in low flow. ρ(total methylmercury) in outflows collected in summer and fall were significantly higher than those sampled in winter and spring. The ρ(methylmercury) increased at several sites below reservoir because of the construction of cascade reservoirs, therefore, it is possible that ρ (methylmercury) would increase dramatically with the development of reservoir. |
来源
|
环境科学研究
,2008,21(2):29-34 【核心库】
|
关键词
|
乌江流域
;
梯级水库
;
甲基汞
;
时空分布
|
地址
|
1.
中国科学院地球化学研究所, 环境地球化学国家重点实验室, 贵州, 贵阳, 550002
2.
贵州大学资源与环境学院, 贵州, 贵阳, 550003
|
语种
|
中文 |
文献类型
|
研究性论文 |
ISSN
|
1001-6929 |
学科
|
环境质量评价与环境监测 |
基金
|
国家自然科学基金
;
中国科学院知识创新工程重要方向项目
|
文献收藏号
|
CSCD:3222147
|
参考文献 共
27
共2页
|
1.
Balogh S J. A comparison of total mercury and methylmereury export from various Minnesota watersheds.
Sei Total Environ,2005,340:261-270
|
CSCD被引
2
次
|
|
|
|
2.
Bonzongo J C. Mercury levels in surface waters of the Carson River-Lahontan Reservoir system Nevada:influence of historic mining activity.
Environ Pollut,1996,92(2):193-201
|
CSCD被引
7
次
|
|
|
|
3.
Canavan C M. Discharge of methylmercury-enriched hypolimnetie water from a stratified reservoir.
Sei Total Environ,2000,260:159-170
|
CSCD被引
12
次
|
|
|
|
4.
Cboe K-Y. Distribution of particulate colloidal and dissolved mercury in San Francisco Bay estuary:2 menomethyl mercury.
Limnology and Oceanography,2003,48:1547-1556
|
CSCD被引
1
次
|
|
|
|
5.
Domagalski J. Occurrence and transport of total mercury and methylmercury in the Sacramento River Basin California.
Journal of Geochemical Exploration,1998,64:277-291
|
CSCD被引
3
次
|
|
|
|
6.
Donkor A K. Mercury in different environmental compartments of the Pra River Basin Ghana.
Sai Total Environ,2006,368:164-176
|
CSCD被引
6
次
|
|
|
|
7.
Eckley C S. Determination of mercury methylation potentials in the water column of lakes across Canada.
Sci Total Environ,2006,368:111-125
|
CSCD被引
16
次
|
|
|
|
8.
Hecky R E. Increased methylmercury contamination in fish in newly formed freshwater reservoirs//Suzuki T.
Advances in mercury toxicology,1991
|
CSCD被引
5
次
|
|
|
|
9.
Heyes A. Methylmercury in pristine and impounded boreal peatlands experimental lakes area Qntario.
Canada Journal of Fish Aquatic Science,2000,57(11):2211-2222
|
CSCD被引
9
次
|
|
|
|
10.
Kelly C A. Increases in fluxes of greenhouse gases and methylmercury following flooding of an experimental reservoir.
Environ Sci Technol,1997,31:1334-1344
|
CSCD被引
34
次
|
|
|
|
11.
Montgomery S. Temporal and spatial influences of flooding on dissolved mercury in boreal reservoirs.
Sci Total Environ,2000,260:147-157
|
CSCD被引
7
次
|
|
|
|
12.
Paller M H. Influence of methylmercury from tributary streams on mercury levels in Savannah River Asiatic clams.
Sci Total Environ,2004,325:209-219
|
CSCD被引
5
次
|
|
|
|
13.
Schetagnc R. Export of mercury downstream from reservoirs.
Sci Total Environ,2000,260:135-145
|
CSCD被引
1
次
|
|
|
|
14.
St Louis V L. The rise and fall of mercury methylation in an experimental reservoir.
Environ Sci Technol,2004,38:1348-1358
|
CSCD被引
13
次
|
|
|
|
15.
Tremblay A. Accumulation of total mercury and methylmercury in insect larvae of hydroelectric reservoirs.
Canada Journal of Fish Aquatic 5cience,1997,54:832-841
|
CSCD被引
6
次
|
|
|
|
16.
Tremblay A. Total mercury and methylmercury accumulation in zooplankton of hydroelectric reservoirs in northern Québec(Canada).
Sci Total Environ,1998,213:307-315
|
CSCD被引
7
次
|
|
|
|
17.
Tremblay A. Total mercury and methylmercury fluxes via emerging insects in recently flooded hydroelectric reservoirs and a natural lake.
Sci Total Environ,1998,219:209-221
|
CSCD被引
10
次
|
|
|
|
18.
Yingcharoen D. Elevated mercury levels in fish resulting from reservoir flooding in Thailand.
Asian Fisheries Science,1993(6):73-80
|
CSCD被引
3
次
|
|
|
|
19.
段水旺.
长江营养元素输送的规律和来源,2000
|
CSCD被引
1
次
|
|
|
|
20.
何天容. 季节性缺氧水库甲基汞的产生及其对下游水体的影响.
湖泊科学,2006,18(6):565-571
|
CSCD被引
12
次
|
|
|
|
|