聚合物固态电解质-锂负极界面的研究进展
Research progress in solid polymer electrolyte- lithium metal anode interface
查看参考文献101篇
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文摘
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固态锂电池是新能源领域最有希望的下一代高能量密度电池体系之一。本文以聚合物固态电解质-锂负极界面的构型特征和形成机理为基础,系统讨论界面接触性、界面化学和电化学反应、锂负极枝晶生长等问题对二者之间的界面稳定性与兼容性的影响。基于此,本文重点阐述了掺杂改性、结构设计等手段在三种聚合物基体与锂负极之间的界面的应用。此外,本文还综述了常见界面表征手段及其在聚合物固态电解质-锂负极界面的应用情况。最后,基于设计和构筑稳定的聚合物固态电解质-锂负极界面的相关策略,本文对掺杂、核层设计等界面优化手段的发展前景进行分析与展望。 |
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其他语种文摘
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Solid state lithium battery is expected to be one of the next generation of battery systems with high energy density in the field of high energy. Based on the constructure characteristics and related formation mechanism of interface between solid polymer electrolyte and lithium anode, the impact of interface contact, interface chemistry and electrochemical reaction, and moreover, the growing process of lithium dendrite and other problems on the interface stability and compatibility were systematically discussed in this review.Thus, the application of doping modification, structure design, and other methods for the interfaces between polymer matrix and lithium anode were also emphasized. In addition, the common interface characterization methods and their applications on the interface between solid polymer electrolyte and lithium anode were also reviewed. Finally, based on the relevant strategies of designing and constructing a stable polymer solid electrolyte-lithium anode interface,the development prospects of interface optimization methods such as doping and core layer design were analyzed and prospected in this paper. |
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来源
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材料工程
,2022,50(5):62-77 【核心库】
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DOI
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10.11868/j.issn.1001-4381.2021.000448
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关键词
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全固态锂电池
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聚合物固态电解质
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锂负极
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固-固界面
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界面修饰
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界面表征
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地址
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广东工业大学材料与能源学院新能源材料与器件系, 广州, 510006
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语种
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中文 |
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文献类型
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综述型 |
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ISSN
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1001-4381 |
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学科
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化学 |
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基金
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国家自然科学基金项目
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广东省科技厅对外合作项目
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珠海市科技创新局产学研合作项目
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文献收藏号
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CSCD:7191375
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