有机胺吸收二氧化碳的热力学和动力学研究进展
A review for research on thermodynamics and kinetics of carbon dioxide absorption with organic amines
查看参考文献116篇
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文摘
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二氧化碳捕集与封存技术(CCS)是针对大气CO_2含量增高导致的全球气候变暖而提出的全球性解决方案。有机胺吸收法作为经济与技术层面最成熟的技术,是实现二氧化碳捕集的重要工艺过程。从有机胺法吸收二氧化碳的基本反应机理出发,系统评述了应用有机胺法吸收捕集CO_2的热力学与动力学性质的研究进展,介绍了不同类型胺溶剂分子结构与CO_2捕集溶解度和反应速度的关系,并对今后CO_2吸收捕集的热力学和动力学的研究方向提出了展望。 |
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其他语种文摘
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Carbon capture and storage technology is aimed to solve the problem of global warming mainly caused by increase of atmospheric CO_2 level. Amine absorption method, as the most mature technology with economic and technical aspects, is an important technology for CO_2 capture. In this review, from the start point of basic reaction mechanism, research works and results on the thermodynamic and kinetic properties of CO_2 absorption with amines are summarized, and relationship of CO_2 absorption solubility and reaction rates with molecular structures of different types of amines are described. Finally some research directions for thermodynamics and kinetics of CO_2 absorption are put forward. |
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来源
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化工学报
,2014,65(1):12-21 【核心库】
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DOI
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10.3969/j.issn.0438-1157.2014.01.002
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关键词
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热力学
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动力学
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CO_2捕集
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吸收法
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有机胺
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地址
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清华大学, 化学工程联合国家重点实验室, 北京, 100084
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语种
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中文 |
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文献类型
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综述型 |
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ISSN
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0438-1157 |
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学科
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化学工业 |
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基金
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国家自然科学基金项目
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中石油专项
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文献收藏号
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CSCD:5033833
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参考文献 共
116
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