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青海湖沉积物中多环芳烃的沉积记录
Historical records of sediment polycyclic aromatic hydrocarbons in Qinghai Lake,Northwest China

查看参考文献27篇

郭建阳 1 *   廖海清 2   张亮 2   汤智 2   吴丰昌 2  
文摘 采用GC/MS方法分析了青海湖沉积柱中16种美国EPA优先控制的多环芳烃(TPAHs)的垂直分布状况,并对其来源进行了分析。研究表明,020 cm沉积柱中TPAHs的含量为495.11172.5 ng.g-1,随沉积年代的更新TPAHs的含量呈增加趋势。这与珠江口和东海沉积柱中的记录基本一致,但明显不同于发达国家同类研究的结果。青海湖沉积物PAHs以23环(包括萘、苊、苊烯、芴、菲和蒽)为主,其含量平均占沉积物中PAHs总量的(72.4±8.9)%。青海湖沉积物中的PAHs主要来自长距离的大气传输,家庭燃煤与木材的低温燃烧是其主要来源,高温燃烧过程释放的PAHs(如机动车尾气的排放)近年来有明显增加的趋势。
其他语种文摘 By adopting GC/MS techniques,this paper analyzed the vertical distribution of 16 priority polycyclic aromatic hydrocarbons(PAHs)proposed by US EPA in a dated 0-20 cm sediment core from Qinghai Lake in Northwest China,and identified the possible sources of the PAHs.The total PAHs(sum of 16 the priority PAHs,TPAHs)concentration in the core ranged from 495.1 to 1172.5 ng.g-1,and had an increasing trend from deeper layer to surface layer.The vertical profile of the sediment PAHs in Qinghai Lake was basically similar to that in the East China Sea and the Pearl River Estuary,but clearly different from that in developed countries.The sediment PAHs in Qinghai Lake were dominated by 2-3 rings PAHs(including naphthalene,acenaphthylene,acenaphthene,fluorene,phenanthrene,and anthracene),accounting for 72.4%±8.9% of TPAHs on an average.The sediment PAHs in Qinghai Lake were mainly originated from the long-distance atmospheric transport resulting from low temperature combustion of domestic coal and woods,but the PAHs from high temperature process(such as vehicle emission)had an obvious increasing trend in recent years.
来源 生态学杂志 ,2011,30(7):1467-1472 【核心库】
关键词 青海湖 ; 沉积柱 ; 多环芳烃 ; 来源
地址

1. 中国科学院地球化学研究所, 环境地球化学国家重点实验室, 贵阳, 550002  

2. 中国环境科学研究院湖泊生态环境研究中心, 国家环境保护湖泊污染国家重点实验室, 北京, 100080

语种 中文
文献类型 研究性论文
ISSN 1000-4890
学科 环境科学基础理论
基金 国家自然科学基金项目 ;  国家973计划 ;  中国科学院西部之光人才培养计划
文献收藏号 CSCD:4261047

参考文献 共 27 共2页

1.  郭建阳. 密云水库沉积物中多环芳烃的垂直分布,来源及生态风险评估. 环境科学,2010,31(3):75-80 被引 1    
2.  王新红. 厦门西港沉积物中多环芳烃的垂直分布特征与污染追踪. 中国环境科学,1997,17(1):19-22 被引 19    
3.  吴莹. 多环芳烃在渤海海峡柱状沉积物中的分布. 环境科学,2001,22(2):74-77 被引 25    
4.  Christensen ER. Source apportionment of PAHs in sediments using factor analysis by time records:Application to Lake Michigan,USA. Water Research,2007,41:168-176 被引 19    
5.  Colombo JC. Sources,vertical fluxes,and equivalent toxicity of aromatic hydrocarbons in coastal sediments of the Rio de la Plata Estuary,Argentina. Environmental Science and Technology,2006,40:734-740 被引 6    
6.  Fernandez P. The historical record of atmospheric pyrolytic pollution over Europe registered in the sedimentary PAH from remote mountain lakes. Environmental Science and Technology,2000,34:1906-1913 被引 17    
7.  Goguo A. Organic aerosols in Eastern Mediterranean:Components source reconciliation by using molecular markers and atmospheric back trajectories Organic Geochemistry. Organic Geochemistry,1996,25:79-96 被引 7    
8.  Gu SH. Source apportionment of PAHs in dated sediments from the Black River,Ohio. Water Research,2003,37:2149-2161 被引 1    
9.  Guo Z. High-resolution depositional records of polycyclic aromatic hydrocarbons in the central continental shelf mud of the East China Sea. Environmental Science and Technology,2006,40:5304-5311 被引 14    
10.  Harrison RM. Source apportionment of atmospheric polycyclic aromatic hydrocarbons collected from an urban location in Birmingham. U.K.Environmental Science and Technology,1996,30:825-832 被引 182    
11.  Ishitake M. Vertical profile of polycyclic aromatic hydrocarbons in a sediment core from a reservoir in Osaka City. Environmental Geology,2007,52:123-129 被引 9    
12.  Kannan K. Spatial and temporal distribution of polycyclic aromatic hydrocarbons in sediments from Michigan inland lakes. Environmental Science and Technology,2005,39:4700-4706 被引 30    
13.  Katsoyiannis A. On the use of PAH molecular diagnostic ratios in sewage sludge for the understanding of the PAH sources.Is this use appropriate. Chemosphere,2007,69:1337-1339 被引 22    
14.  Li K. PAHs in dated sediments of ashtabula river,Ohio,USA. Environmental Science and Technology,2001,35:2896-2902 被引 9    
15.  Lima ALC. High-resolution record of pyrogenic polycyclic aromatic hydrocarbon deposition during the 20 th Century. Environmental Science and Technology,2003,37:53-61 被引 16    
16.  Liu GQ. Sedimentary record of polycyclic aromatic hydrocarbons in a sediment core from the Pearl River Estuary,South China. Marine Pollution Bulletin,2005,51:912-921 被引 29    
17.  Mai BX. Distribution of polycyclic aromatic hydrocarbons in the coastal region off Macao,China:Assessment of input sources and transport pathways using compositional analysis. Environmental Science and Technology,2003,37:4855-4863 被引 88    
18.  Masclet P. Evidence for the presence of polycyclic aromatic hydrocarbons in the polar atmosphere and in the polar ice of Greenland. Analusis,1995,23:250-252 被引 3    
19.  Miguel AH. Benzo[k]fuoranthene,benzo[ghi] perylene,and indeno[1,2,3-cd] pyrene:New tracers of automotive emissions in receptor modeling. Aerosol Science and Technology,1989,10:292-295 被引 21    
20.  Rose NL. The historical record of PAH,PCB,trace metal and fly-ash particle deposition at a remote lake in north-west Scotland. Environmental Pollution,2002,117:121-132 被引 7    
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