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改性生物炭对水体中抗生素的去除研究进展
Research progress on the removal of antibiotics in water by modified biochar

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蒋宗宏 1   陈淼 1,2,3   李心清 4   冯乾伟 1   王兵 1,2,3 *  
文摘 随着社会经济的不断发展,抗生素造成的水体环境污染问题已不容忽视.利用生物炭去除水体中的抗生素是解决这一问题的有效手段之一.然而,原始生物炭对水体中抗生素等有机污染物的去除存在一定局限性,因此对生物炭进行改性以提升其吸附能力尤为必要.生物炭的吸附性能受生物质类型、碳化条件和改性方法等因素影响较大,导致目前虽然开展了许多相关研究,但结论不一,尤其是在不同改性生物炭对不同抗生素吸附机理的解释方面还不是很清楚,因此有必要对现有研究进行系统地归纳和总结.本文首先对用于抗生素吸附的改性生物炭制备方法及理化性质表征方法进行了介绍,综述了改性生物炭对不同种类抗生素(磺胺类、喹诺酮类、四环素类、大环内酯类、氯霉素类)的吸附效果、吸附机理及其影响因素(如溶液pH值、热解温度、改性材料等),对比分析了生物炭改性前后吸附效果的差异,对目前改性生物炭用于去除水体中抗生素存在的问题进行了分析和总结,在此基础上,对今后该领域的研究和发展方向进行了展望,以期为将来开展相关的研究工作提供一定的参考.
其他语种文摘 With the constant development of the social economy, the water pollution caused by antibiotics have already become serious. Removing antibiotics from water through the biochar is an effective solution to the problem. However, there are some limitations about the removal of antibiotics and other organic pollutants by the pristine biochar, so it is necessary to modify the biochar so as to improve its adsorption capacity. The adsorption capacity of the biochar is greatly related to biomass types, carbonization conditions and modification methods. As a result, although a lot of related research have been carried out, there are different conclusions, especially the obscure explanation of the adsorption mechanisms on various antibiotics by different modified biochar. Therefore, it is necessary to systematically summarize the current research results. Firstly, the preparation and physicochemical characterization methods of the modified biochar for antibiotic adsorption are introduced. The adsorption effects, adsorption mechanisms and influencing factors (such as solution pH value, pyrolysis temperature and modified material) of different kinds of antibiotics (sulfonamides, quinolones, tetracyclines, macrolides and chloramphenicols) are reviewed. The difference of the adsorption effect before and after biochar modification is analyzed and summarized. On this basis, suggestions and future perspectives are proposed, providing a reference for future research.
来源 环境化学 ,2021,40(12):3846-3860 【核心库】
DOI 10.7524/j.issn.0254-6108.2020080202
关键词 改性生物炭 ; 抗生素 ; 吸附机理 ; 污水处理
地址

1. 贵州大学资源与环境工程学院, 贵阳, 550025  

2. 喀斯特地质资源与环境教育部重点实验室, 喀斯特地质资源与环境教育部重点实验室, 贵阳, 550025  

3. 贵州喀斯特环境生态系统教育部野外科学观测研究站, 贵州喀斯特环境生态系统教育部野外科学观测研究站, 贵阳, 550025  

4. 中国科学院地球化学研究所, 环境地球化学国家重点实验室, 贵阳, 550081

语种 中文
文献类型 研究性论文
ISSN 0254-6108
学科 行业污染、废物处理与综合利用
基金 国家重点研发计划项目 ;  国家自然科学基金 ;  贵州省高层次留学人才创新创业择优资助项目 ;  贵州大学自然科学专项(特岗)科研基金项目
文献收藏号 CSCD:7139208

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引证文献 3

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CSCD被引 4

2 牛经纬 农业固废生物炭及其改性材料对重金属的吸附研究 工业水处理,2023,43(12):26-35
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