利用薄膜扩散梯度技术估算红枫湖沉积物磷释放通量
Estimation of the Phosphorus Flux from the Sediment of Hongfeng Lake Using the Zr-Oxide Diffusive Gradient in Thin Films (Zr-Oxide DGT) Technique
查看参考文献34篇
文摘
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湖水因季节性分层而导致底层滞水带缺氧的亚深水型湖泊,其沉积物内源磷释放对水体磷循环和富营养化有着重要影响。选取典型的高原亚深水型湖泊———贵州红枫湖为研究对象,借助氧化锆薄膜扩散梯度技术获取了5个代表性湖区沉积物有效磷(labile P)的原位、二维、高分辨分布信息,在此基础上估算夏季红枫湖沉积物内源磷释放通量。结果表明,红枫湖后五沉积物有效磷浓度最高,羊昌河、大坝次之,南湖中与北湖中较低。红枫湖沉积物labile P浓度在亚毫米水平上有很大差异,空间分布不均一,时间上夏季磷释放量为6270~ 7999 kg,占全湖水体总磷的22% ~ 28%。沉积物磷释放是红枫湖水体磷的重要来源,在湖泊富营养化防治过程中应予以重视。 |
其他语种文摘
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Phosphorus(P) released from sediments has a great effect on the lake eutrophication,especially in the deep-water lakes. In this study,in situ two-dimensional,high-resolution distribution of labile P in sediments from five typical lake areas in the Hongfeng lake,a typical sub-deep lake,were characterized using the Zr-oxide diffusive gradients in thin films (DGT) technique,and the P flux in a summer time was accurately estimated. Our results showed that the labile P concentration in Houwu was the highest among five areas of the lake. Concentrations of labile P in sediments of Yangchang and Dam areas were slightly lower than that of Houwu,and the Mid-north and Mid-south areas have the lowest labile P concentrations. The distribution of labile P exhibited large heterogeneity at the sub-millimeter spatial resolution. The calculated P flux based on the diffusion model ranged from 6270 kg to 7999 kg,accounting for 22% to 28% of the total P of the water. Thus,the internal P is an important source for water P in the Hongfeng lake and should be taken seriously in the management of eutrophication. |
来源
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矿物岩石地球化学通报
,2015,34(5):1014-1020 【核心库】
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DOI
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10.3969/j.issn.1007-2802.2015.05.017
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关键词
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红枫湖
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沉积物
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Zr-oxide DGT
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磷
;
高分辨率
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地址
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1.
贵州大学资源与环境工程学院, 环境地球化学国家重点实验室, 贵阳, 550025
2.
中国科学院地球化学研究所, 环境地球化学国家重点实验室, 贵阳, 550002
3.
中国科学院南京地理与湖泊研究所, 湖泊与环境国家重点实验室, 南京, 210008
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语种
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中文 |
文献类型
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研究性论文 |
ISSN
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1007-2802 |
学科
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地质学 |
基金
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国家科技支撑计划项目
;
国家自然科学基金项目
;
贵州省项目
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文献收藏号
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CSCD:5581880
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参考文献 共
34
共2页
|
1.
Bennett W W. New diffusive gradients in a thin film technique for measuring inorganic arsenic and selenium(Ⅳ) using a titanium dioxide based adsorbent.
Analytical Chemistry,2010,82(17):7401-7407
|
CSCD被引
10
次
|
|
|
|
2.
Burger D F. Benthic nutrient fluxes in a eutrophic,polymictic lake.
Hydrobiologia,2007,584(1):13-25
|
CSCD被引
10
次
|
|
|
|
3.
Carpenter S R. Phosphorus control is critical to mitigating eutrophication.
Processings of the National Academy of Sciences of the United States of America,2008,105(32):11039-11040
|
CSCD被引
61
次
|
|
|
|
4.
Chen H. Effective concentration difference model to study the effect of various factors on the effective diffusion coefficient in the dialysis membrane.
Analytica Chimica Acta,2011,698(1/2):27-35
|
CSCD被引
8
次
|
|
|
|
5.
Chen J A. Time and spatial distribution characteristics of nitrogen and phosphorus in the sediment of Lake Hongfeng.
13th World Lake Conference,2009:2226-2230
|
CSCD被引
3
次
|
|
|
|
6.
Davison W. In-situ speciation measurements of trace components in natural-water using thin-film gels.
Nature,1994,367(6463):546-548
|
CSCD被引
92
次
|
|
|
|
7.
Ding S M. Gel-based coloration technique for the submillimeter-scale imaging of labile phosphorus in sediments and soils with diffusive gradients in thin films.
Environment Science & Technology,2013,47(14):7821-7829
|
CSCD被引
12
次
|
|
|
|
8.
Ding S M. Development of the DET technique for high-resolution determination of soluble reactive phosphate profiles in sediment pore waters.
International Journal of Environmental Analytical Chemistry,2010,90(14/15):1130-1138
|
CSCD被引
13
次
|
|
|
|
9.
Ding S M. Measurement of dissolved reactive phosphorus using the diffusive gradients in thin films technique with a high-capacity binding phase.
Environment Science & Technology,2010,44(21):8169-8174
|
CSCD被引
21
次
|
|
|
|
10.
Ding S M. High-resolution simultaneous measurements of dissolved reactive phosphorus and dissolved sulfide: The first observation of their simultaneous release in sediments.
Environment Science & Technology,2012,46(15):8297-8304
|
CSCD被引
18
次
|
|
|
|
11.
Eggleton J. A review of factors affecting the release and bioavailability of contaminants during sediment disturbance events.
Environment International,2004,30(7):973-980
|
CSCD被引
65
次
|
|
|
|
12.
Elsbury K E. Using oxygen isotopes of phosphate to trace phosphorus sources and cycling in Lake Erie.
Environment Science & Technology,2009,43(9):3108-3114
|
CSCD被引
19
次
|
|
|
|
13.
Menzies N W. Assessment of P availability in heavily fertilized soils using the diffusive gradient in thin films(DGT) technique.
Plant and Soil,2005,269(1/2):1-9
|
CSCD被引
5
次
|
|
|
|
14.
Monbet P. Combined gel probes for the in situ determination of dissolved reactive phosphorus in porewaters and characterization of sediment reactivity.
Environment Science & Technology,2008,42(14):5112-5117
|
CSCD被引
10
次
|
|
|
|
15.
Ozkundakci D. Hypolimnetic phosphorus and nitrogen dynamics in a small,eutrophic lake with a seasonally anoxic hypolimnion.
Hydrobiologia,2011,661(1):5-20
|
CSCD被引
16
次
|
|
|
|
16.
Pichette C. Using diffusive gradients in thinfilms for in situ monitoring of dissolved phosphate emissions from freshwater aquaculture.
Aquaculture,2009,286(3/4):198-202
|
CSCD被引
1
次
|
|
|
|
17.
Santner J. High-resolution chemical imaging of labile phosphorus in the rhizosphere of Brassica napus L. cultivars.
Environmental and Experimental Botany,2012,77:219-226
|
CSCD被引
8
次
|
|
|
|
18.
Seiki T. Benthic nutrient remineralization and oxygen consumtion in the coastal area of Hiroshima Bay.
Water Resources,1989,23(2):219-228
|
CSCD被引
35
次
|
|
|
|
19.
Sondergaard M. Role of sediment and internal loading of phosphorus in shallow lakes.
Hydrobiologia,2003,506/509(1/3):135-145
|
CSCD被引
143
次
|
|
|
|
20.
Stockdale A. High-resolution twodimensional quantitative analysis of phosphorus,vanadium and arsenic,and qualitative analysis of sulfide,in a freshwater sediment.
Environmental Chemistry,2008,5(2):143-149
|
CSCD被引
10
次
|
|
|
|
|