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Synthesis of flower-like α-Fe_2O_3 and its application in wastewater treatment
花状氧化铁的制备及其在废水处理中的应用

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文摘 The removal of arsenic from aqueous solution is crucial to human health and environmental pollution. Herein, flower-like α-Fe_2O_3 nanostructures were synthesized via a template-free microwave-assisted solvothermal technique, and were applied as adsorbents for the removal of arsenic (As(V)) from aqueous solutions. The results indicated that the synthesized flower-like α-Fe_2O_3 showed excellent sorption properties and had a maximum sorption capacity of 47.64 mg/g for As(V). Meanwhile, the experimental results of photodegradation of methylene blue (MB) indicated that the as-synthesized flower-like α-Fe_2O_3 exhibited very high photocatalytic performance for the photodegradation of MB and that the as-obtained flower-like α-Fe_2O_3 nanostructures were suitable materials in wastewater treatment.
其他语种文摘 研究目的:研究花状氧化铁的制备并探讨其对砷的吸附性能和亚甲基蓝的催化性能。创新要点:1. 合成了花状氧化铁;2. 发现Langmuir 模型能更好地模拟砷的吸附过程;3. 发现花状氧化铁对亚甲基蓝有很好的催化降解性能。研究方法:1. 使用扫描电镜、投射电镜、X 射线衍射和BET 比表面及孔径分析仪对合成的花状氧化铁进行表征;2. 采用静态实验法研究砷的吸附性能及亚甲基蓝的催化行为。重要结论:1. 采用一种低成本的溶剂热法合成了花状氧化铁;2. 合成的花状氧化铁有着较大的比表面积并对砷有着很好的吸附性能,并且吸附率随着pH 的增加而降低。同时发现Langmuir 模型能更好地模拟砷的吸附过程;3. 亚甲基蓝的初始浓度和花状氧化铁的用量对催化性能影响较为明显,花状氧化铁有较好的重复利用性;4. 合成的花状氧化铁可以应用于大批废水的处理。
来源 Journal of Zhejiang University. Science A , Applied Physics & Engineering,2014,15(8):671-680 【核心库】
DOI 10.1631/jzus.a1400133
关键词 Flower-like α-Fe_2O_3 ; Arsenate ; Sorption ; Methylene blue (MB) ; Photodegradation
地址

1. Chongqing Three Gorges University, Key Laboratory of Water Environment Evolution and Pollution Control in Three Gorges Reservoir, Chongqing, 404100  

2. Institute of Plasma Physics, Chinese Academy of Sciences, Hefei, 230031  

3. NAAM Research Group, Department of Mathematics, Faculty of Science, King Abdulaziz University, Saudi Arabia, Jeddah, 21589

语种 英文
文献类型 研究性论文
ISSN 1673-565X
学科 环境污染及其防治
基金 国家自然科学基金 ;  the Natural Science Foundation of Chongqing Science & Technology Commission
文献收藏号 CSCD:5215247

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引证文献 4

1 Yang Kun Environmental risks of engineered nanomaterials Journal of Zhejiang University. Science A, Applied Physics & Engineering,2014,15(8):547-551
被引 2

2 杜毅 人工纳米材料吸附放射性核素的机理研究 农业环境科学学报,2016,35(10):1837-1847
被引 5

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